I can recommend
Almagro (<-nice site but in Spanish) We spent a night there on our way down to Sevilla for Semana Santa. They have the oldest theater in Spain,
a NICE, BIG square with some fountains, statues, and palms. Walking the old streets made me think of Colonial Spain in Latin America. VERY nice.
Aranjuez is pretty cool too, though, with its palace, VERY romantic gardens & fountains, and a nice little town too:
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